Application of high specific surface area Ag/AgCl/TiO2 coupled photocatalyst fabricated by fused filament fabrication
學年 110
學期 2
出版(發表)日期 2022-03-17
作品名稱 Application of high specific surface area Ag/AgCl/TiO2 coupled photocatalyst fabricated by fused filament fabrication
作品名稱(其他語言)
著者 Lin, Ching‑bin
單位
出版者
著錄名稱、卷期、頁數 The International Journal of Advanced Manufacturing Technology 120, p.4539-4550
摘要 This study used a three-dimensional (3D) printing process to develop the Ag/AgCl/TiO2 coupled photocatalyst with a specific surface area of 748 mm2/g. We examined the catalytic capability of this photocatalyst in degrading methyl blue (MB) dye and sterilizing Escherichia coli as well as the durability and reliability of its continuous use. A TiO2 module was constructed through fused filament fabrication (FFF), and the adopted 3D printing filament was composed of anatase TiO2 nanoparticles, stearic acid, wax, and a plasticizer. The green compact of the TiO2 module was subjected to solvent debinding, thermal debinding, and sintering to obtain a fundamental structure that was subsequently coupled with AgCl through a precipitation reaction. Ultraviolet radiation was used for the photoreduction to obtain the Ag/AgCl/TiO2 coupled photocatalyst coupling module. This photocatalyst can effectively degrade MB dye and disinfect E. coli. The degradation of MB dye and sterilization of E. coli were conducted under visible and ultraviolet light. The degradation of MB dye by the Ag/AgCl/TiO2 coupled photocatalyst was a first-order reaction. In addition, this coupled photocatalyst could retain its MB dye degradation rate (95%) for five cycles. E. coli was sterilized using the prepared photocatalytic module in a 120-min test, and this sterilization phenomenon could be presented as a hyperbolic reaction. The photocatalytic module manufactured in this study through FFF could efficiently degrade pollutants in water, and its durability and reliability after repeated use have been approved.
關鍵字 Silver chloride;Fused filament fabrication;Methyl blue dye;Escherichia coli;Reliability
語言 en
ISSN 1433-3015
期刊性質 國外
收錄於 SCI
產學合作
通訊作者
審稿制度
國別 GBR
公開徵稿
出版型式 ,電子版,紙本
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