High-pressure electrocoagulation system with periodic air replenishment for efficient dye wastewater treatment: Reaction dynamics and cost evaluation
學年 107
學期 2
出版(發表)日期 2019-03-10
作品名稱 High-pressure electrocoagulation system with periodic air replenishment for efficient dye wastewater treatment: Reaction dynamics and cost evaluation
作品名稱(其他語言)
著者 Ya, Vinh; Martin, Natacha; Choo, Kwang-Ho; Chou, Yi-Hsuan; Lee, Shou-Jen; Le, Ngoc Chung; Li, Chi-Wang
單位
出版者
著錄名稱、卷期、頁數 Journal of Cleaner Production 213, p.1127-1134
摘要 Ferrous ions are the major Fe species generated from sacrificial iron anodes, but ferric ions are the more active ingredients for the removal of organic matters in the acidic pH region. Therefore, a novel high-pressure electrocoagulation (HPEC) system was devised to facilitate the Fe(II)-to-Fe(III) conversion under acidic pH conditions. The effects of operation pressure (0–3 bar) and initial pH value (3–10) on the removal of color and organics from synthetic dye wastewater containing Eriochrome Black T (EBT) were investigated. The operation costs of the HPEC were compared with that of the conventional electrocoagulation (CEC) processes. The HPEC outperformed the CEC, achieving complete color removal after a short reaction time. In the initial pH range of <8, the HPEC achieved substantial color (∼100%) and organic carbon (∼78%) removals. However, a sharp drop in the removal efficiency occurred at the pH of >8 owing to the formation of Fe(III)-EBT complexes and the ineffective removal of these complexes by coagulation or adsorption. The high removal efficiencies attained under acidic and neutral pH conditions were attributed to the effective Fe(II)-to-Fe(III) conversion by dissolved oxygen under pressure followed by the formation of Fe(OH)3 precipitates. The HPEC saves significant operating costs (45–70%) compared to the CEC process.
關鍵字 Intermittent air replenishment;Electrocoagulation;Economic evaluation;Fe species;High-pressure system
語言 en_US
ISSN
期刊性質 國外
收錄於 SCI EI
產學合作
通訊作者 Chi-Wang Li
審稿制度
國別 GBR
公開徵稿
出版型式 ,電子版
相關連結

機構典藏連結 ( http://tkuir.lib.tku.edu.tw:8080/dspace/handle/987654321/115724 )