標題:Highly robust and efficient Ti-based Sb-SnO2 anode with a mixed carbon and nitrogen interlayer for electrochemical 1,4-dioxane removal from water |
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學年 | 109 |
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學期 | 1 |
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出版(發表)日期 | 2020/08/01 |
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作品名稱 | Highly robust and efficient Ti-based Sb-SnO2 anode with a mixed carbon and nitrogen interlayer for electrochemical 1,4-dioxane removal from water |
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作品名稱(其他語言) | |
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著者 | Naresh Mameda; Hyeona Park; Syed Salman Ali Shah; Kibaek Lee; Chi-Wang Li; Vincenzo Naddeo; Kwang-Ho Choo |
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單位 | |
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出版者 | |
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著錄名稱、卷期、頁數 | Chemical Engineering Journal 393, 124794 |
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摘要 | Ti-based Sb-SnO2 electrodes are attractive due to their excellent catalytic activity but have a short service life. Here, we report a highly stable and efficient Ti/TiONC/Sb-SnO2 electrode, which was fabricated through hydrothermal reactions using urea to form TiONC interlayers and electrodeposition-annealing to coat the active Sb-SnO2 catalysts. The triple-layered anode was characterized by highly crystalline structures, high oxygen evolution potentials, and corrosion-resistance properties. The structural arrangement yielded better electrocatalytic performances than that using the control electrode (Ti/Sb-SnO2), showing enhanced organics degradation efficiencies. This new electrode’s lifetime was significantly (~25 times) longer than that of either the control or any Sb-SnO2 electrode modified with non-precious materials reported in the literature. The electrode’s enhanced stability was attributed to the insertion of the mixed C and N interlayers that are resistant to oxidants and corrosive ions. The Ti/TiONC/Sb-SnO2 anode holds promise for use in electrochemical water treatment. |
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關鍵字 | Sb-SnO2;{4};Interlayer;Service life;1,4-Dioxane |
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語言 | 英文(美國) |
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ISSN | 1873-3212 |
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期刊性質 | 國外 |
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收錄於 | SCI; |
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產學合作 | |
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通訊作者 | |
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審稿制度 | 是 |
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國別 | 荷蘭 |
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公開徵稿 | |
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出版型式 | ,電子版 |
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相關連結 | |
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