Recovery of deuterium from H-D gas mixture in thermal diffusion columns connected in series with countercurrent-flow transverse sampling streams
學年 104
學期 2
出版(發表)日期 2016-07-06
作品名稱 Recovery of deuterium from H-D gas mixture in thermal diffusion columns connected in series with countercurrent-flow transverse sampling streams
作品名稱(其他語言)
著者 Chii-Dong Ho; Ho-Ming Yeh; Ching-Chun Hsu
單位
出版者
著錄名稱、卷期、頁數 International Journal of Hydrogen Energy 41(25), p.10819–10826
摘要 The equations for predicting the degrees of separation of H2, HD and D2 from H–D gas mixture by thermal diffusion in countercurrent-flow concentric-tube Frazier schemes of single and multiple columns, have been derived. The equations for predicting the recovery of deuterium (D) in HD and D2 were then obtained with the use of the atomic weight ratio. The degrees of separation, as well as separation factors, for deuterium recovery in the cryogenic-wall thermal diffusion devices were estimated, with the use of the experimental data obtained by Arita et al., 1998 and with the transport coefficients correlated in the previous work. Considerable improvement in deuterium recovery is achievable if a Frazier scheme with multiple columns is employed, instead of using the single-column device, either with the same column height, or with the same total sum of column heights, especially for the operation under larger volume flow rate and/or higher operating pressure. Further, countercurrent-flow operation is better than concurrent-flow operation in multi-column devices.
關鍵字 Deuterium recovery;H–D gas mixture;Thermal diffusion;Frazier scheme;Countercurrent-flow
語言 en
ISSN 0360-3199
期刊性質 國外
收錄於 SCI EI
產學合作
通訊作者 Chii-Dong Ho
審稿制度
國別 GBR
公開徵稿
出版型式 ,紙本
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