期刊論文
| 學年 | 111 |
|---|---|
| 學期 | 1 |
| 出版（發表）日期 | 2023-01-01 |
| 作品名稱 | Confined Fe single atomic sites on (100) plane of anatase TiO2 nanofibers boost white LED driven Fenton-like norfloxacin degradation |
| 作品名稱（其他語言） | |
| 著者 | Zhilin Ji; Rongsheng Cai; Wanneng Ye; Ping Lu; Chung-Li Dong; Yu-Cheng Huang; Xilin She; Denys S. Butenko; Yiming Liu; Yukun Zhu; Dongjiang Yang |
| 單位 | |
| 出版者 | |
| 著錄名稱、卷期、頁數 | Journal of Cleaner Production 382, 135161 |
| 摘要 | Developing efficient and sustainable photocatalyst is crucial for antibiotic degradation in water treatment. Iron (Fe) species modified semiconductor photocatalysts have been widely used in visible-light driven Fenton-like systems. However, the limited dispersion of Fe sites and low redox rate of the Fe(III)/Fe(II) restrict the catalytic performance. Herein, the atomic Fe sites with highly dispersed coordination centers were confined (100) facets exposed titania nanofibers (Fe-TNFs) for efficient photocatalytic Fenton-like norfloxacin (NOR) degradation. The optimized Fe-TNFs catalyst could achieve 95% NOR removal after 5 h of white LED illumination, which is 15% higher than that of nanostructured Fe species. The high performance is credited for the enhanced visible light absorption, and the efficient electron transfer through Fe–O bonds in Fe-TNFs enables the fast cyclic transformation of Fe(III)/Fe(II), which can promote the continuous production of •OH in the photocatalytic Fenton-like system. This study can provide technical support for the developing a feasible and sustainable wastewater treatment solution, and provide reference for the fate and risk assessment of antibiotics in the environment. |
| 關鍵字 | |
| 語言 | en |
| ISSN | 0959-6526; 1879-1786 |
| 期刊性質 | 國外 |
| 收錄於 | SCI |
| 產學合作 | |
| 通訊作者 | |
| 審稿制度 | 否 |
| 國別 | NLD |
| 公開徵稿 | |
| 出版型式 | ,電子版 |
| 相關連結 |
機構典藏連結 ( http://tkuir.lib.tku.edu.tw:8080/dspace/handle/987654321/125738 ) |