期刊論文
學年 | 107 |
---|---|
學期 | 2 |
出版(發表)日期 | 2019-03-10 |
作品名稱 | High-pressure electrocoagulation system with periodic air replenishment for efficient dye wastewater treatment: Reaction dynamics and cost evaluation |
作品名稱(其他語言) | |
著者 | Ya, Vinh; Martin, Natacha; Choo, Kwang-Ho; Chou, Yi-Hsuan; Lee, Shou-Jen; Le, Ngoc Chung; Li, Chi-Wang |
單位 | |
出版者 | |
著錄名稱、卷期、頁數 | Journal of Cleaner Production 213, p.1127-1134 |
摘要 | Ferrous ions are the major Fe species generated from sacrificial iron anodes, but ferric ions are the more active ingredients for the removal of organic matters in the acidic pH region. Therefore, a novel high-pressure electrocoagulation (HPEC) system was devised to facilitate the Fe(II)-to-Fe(III) conversion under acidic pH conditions. The effects of operation pressure (0–3 bar) and initial pH value (3–10) on the removal of color and organics from synthetic dye wastewater containing Eriochrome Black T (EBT) were investigated. The operation costs of the HPEC were compared with that of the conventional electrocoagulation (CEC) processes. The HPEC outperformed the CEC, achieving complete color removal after a short reaction time. In the initial pH range of <8, the HPEC achieved substantial color (∼100%) and organic carbon (∼78%) removals. However, a sharp drop in the removal efficiency occurred at the pH of >8 owing to the formation of Fe(III)-EBT complexes and the ineffective removal of these complexes by coagulation or adsorption. The high removal efficiencies attained under acidic and neutral pH conditions were attributed to the effective Fe(II)-to-Fe(III) conversion by dissolved oxygen under pressure followed by the formation of Fe(OH)3 precipitates. The HPEC saves significant operating costs (45–70%) compared to the CEC process. |
關鍵字 | Intermittent air replenishment;Electrocoagulation;Economic evaluation;Fe species;High-pressure system |
語言 | en_US |
ISSN | |
期刊性質 | 國外 |
收錄於 | SCI EI |
產學合作 | |
通訊作者 | Chi-Wang Li |
審稿制度 | 否 |
國別 | GBR |
公開徵稿 | |
出版型式 | ,電子版 |
相關連結 |
機構典藏連結 ( http://tkuir.lib.tku.edu.tw:8080/dspace/handle/987654321/115724 ) |